I love SMG, but...no. Her career became troubled when Scooby-Doo 2 was her first post-Buffy flick. The Grudge was even a surprise hit to her own talent agent, and she made a string of unreleased/straight-to-DVD films from 2005 until Ringer hit The CW. She never quite managed to rise above genre films--teen, family, and then horror--or forge her own screen persona outside of "Buffy Summers".
As for Katie, her career was in this weird transition stage post-DC, where her acting was critically acclaimed, but her film roles weren't strong enough to push her into the A-list (they were either indie, or she was secondary lead, or it was a flop mainstream film). If she hadn't hooked up with Tom, there is a chance she could have had, say, Anne Hathaway's career, but now we'll never know because her fame as Tom's wife/ex-wife/Scientologist escapee overshadows her acting.
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